全文获取类型
收费全文 | 32869篇 |
免费 | 2625篇 |
国内免费 | 1254篇 |
专业分类
电工技术 | 1744篇 |
技术理论 | 1篇 |
综合类 | 1993篇 |
化学工业 | 5473篇 |
金属工艺 | 1710篇 |
机械仪表 | 2225篇 |
建筑科学 | 2641篇 |
矿业工程 | 1050篇 |
能源动力 | 858篇 |
轻工业 | 2020篇 |
水利工程 | 557篇 |
石油天然气 | 2137篇 |
武器工业 | 230篇 |
无线电 | 3908篇 |
一般工业技术 | 3994篇 |
冶金工业 | 1606篇 |
原子能技术 | 386篇 |
自动化技术 | 4215篇 |
出版年
2024年 | 62篇 |
2023年 | 574篇 |
2022年 | 719篇 |
2021年 | 1222篇 |
2020年 | 931篇 |
2019年 | 849篇 |
2018年 | 938篇 |
2017年 | 993篇 |
2016年 | 868篇 |
2015年 | 1206篇 |
2014年 | 1565篇 |
2013年 | 1877篇 |
2012年 | 2023篇 |
2011年 | 2137篇 |
2010年 | 1874篇 |
2009年 | 1851篇 |
2008年 | 1690篇 |
2007年 | 1706篇 |
2006年 | 1854篇 |
2005年 | 1657篇 |
2004年 | 1072篇 |
2003年 | 968篇 |
2002年 | 941篇 |
2001年 | 811篇 |
2000年 | 906篇 |
1999年 | 964篇 |
1998年 | 802篇 |
1997年 | 696篇 |
1996年 | 681篇 |
1995年 | 533篇 |
1994年 | 447篇 |
1993年 | 327篇 |
1992年 | 260篇 |
1991年 | 204篇 |
1990年 | 152篇 |
1989年 | 116篇 |
1988年 | 93篇 |
1987年 | 47篇 |
1986年 | 35篇 |
1985年 | 24篇 |
1984年 | 19篇 |
1983年 | 12篇 |
1982年 | 22篇 |
1981年 | 13篇 |
1980年 | 3篇 |
1979年 | 2篇 |
1959年 | 2篇 |
排序方式: 共有10000条查询结果,搜索用时 31 毫秒
1.
Hua Yang Shi-Xiao Wei Han Chen Lang Chen Chak-Tong Au Ting-Liang Xie Shuang-Feng Yin 《American Institute of Chemical Engineers》2022,68(10):e17810
A high-throughput (105.5 g/h) passive four-stage asymmetric oscillating feedback microreactor using chaotic mixing mechanism was developed to prepare aggregated Barium sulfate (BaSO4) particles of high primary nanoparticle size uniformity. Three-dimensional unsteady simulations showed that chaotic mixing could be induced by three unique secondary flows (i.e., vortex, recirculation, and oscillation), and the fluid oscillation mechanism was examined in detail. Simulations and Villermaux–Dushman experiments indicate that almost complete mixing down to molecular level can be achieved and the prepared BaSO4 nanoparticles were with narrow primary particle size distribution (PSD) having geometric standard deviation, σg, less than 1.43 when the total volumetric flow rate Qtotal was larger than 10 ml/min. By selecting Qtotal and reactant concentrations, average primary particle size can be controlled from 23 to 109 nm as determined by microscopy. An average size of 26 nm with narrow primary PSD (σg = 1.22) could be achieved at Qtotal of 160 ml/min. 相似文献
2.
3.
Lu Huaiqian Shi Hui Xie Qilong Li Li Xiao Yong Jia Litao Li Debao 《Catalysis Letters》2022,152(11):3347-3353
Catalysis Letters - This study proposed a new facile route to rational creating oxygen-vacancy (Vo)-rich surface of Co3O4 nanosheets by acetic acid leaching. The acid leached Co3O4 nanosheets was... 相似文献
5.
6.
Christopher J. Marvel Qirong Yang Scott D. Walck Kelvin Y. Xie Kristopher D. Behler Jerry C. LaSalvia Masashi Watanabe Richard A. Haber Martin P. Harmer 《Journal of the American Ceramic Society》2022,105(5):2990-3007
Compositional analysis of boron carbide on nanometer length scales to examine or interpret atomic mechanisms, for example, solid-state amorphization or grain-boundary segregation, is challenging. This work reviews advancements in high-resolution microanalysis to characterize multiple generations of boron carbide. First, ζ-factor microanalysis will be introduced as a powerful (scanning) transmission electron microscopy ((S)TEM) analytical framework to accurately characterize boron carbide. Three case studies involving the application of ζ-factor microanalysis will then be presented: (1) accurate stoichiometry determination of B-doped boron carbide using ζ-factor microanalysis and electron energy loss spectroscopy, (2) normalized quantification of silicon grain-boundary segregation in Si-doped boron carbide, and (3) calibration of a scanning electron microscope X-ray energy-dispersive spectroscopy (XEDS) system to measure compositional homogeneity differences of B/Si-doped arc-melted boron carbides in the as-melted and annealed conditions. Overall, the improvement and application of advanced analytical tools have helped better understand processing–microstructure–property relationships and successfully manufacture high-performance ceramics. 相似文献
7.
最近,存算一体(IMC)架构引起了广泛关注,并被认为有望成为突破冯诺依曼瓶颈的新型计算机架构,特别是在数据密集型(data-intensive)计算中能够带来显著的性能和功耗优势.其中,基于SRAM的IMC架构方案也被大量研究与应用.该文在一款基于SRAM的通用存算一体架构平台——DM-IMCA的基础上,探索IMC架构在物联网领域中的应用价值.具体来说,该文选取了物联网中包括信息安全、二值神经网络和图像处理在内的多个轻量级数据密集型应用,对算法进行分析或拆分,并将关键算法映射到DM-IMCA中的SRAM中,以达到加速应用计算的目的.实验结果显示,与基于传统冯诺依曼架构的基准系统相比,利用DM-IMCA来实现物联网中的轻量级计算密集型应用,可获得高达24倍的计算加速比. 相似文献
8.
9.
Yang Lu Panpan Li Wenqing Xie Yongmin Duan Xiyang Wang Shiqing Xu Junjie Zhang 《Journal of the European Ceramic Society》2021,41(6):3635-3642
Halide perovskite glass-ceramic has recently moved into the center of the attention of perovskite research due to their potential for temperature sensing. However, quantum dots glass-ceramic with excellent luminescence performance still needs to be combined with rare-earth (RE) ions to accurately measure temperature. In this work, a novel non-RE doped dual-emission (460 nm and 512 nm) CsPbBr3 quantum dots was obtained in telluride glass via the friction crystallization method, where 512 nm was derived from intrinsic luminescence of quantum dots, and 460 nm was originated from thermally induced bromine vacancy, which can be used for temperature sensing. Fluorescence intensity ratio results indicate that the relative sensitivity of dual-emission could reach 5.6 % K?1 at 323 K. The discovery of non-RE doped CsPbBr3 QDs glass-ceramic with negative thermal quenching uncovers a new optional sensing glass material that surpass traditional RE-doped QDs glass by their tunability and sensitivity. 相似文献
10.
Hengtao Wang Hui Chen Weicheng Xie Hanjian Lai Tingxing Zhao Yulin Zhu Lin Chen Chunxian Ke Nan Zheng Feng He 《Advanced functional materials》2021,31(26):2100877
The design of polymer acceptors plays an essential role in the performance of all-polymer solar cells. Recently, the strategy of polymerized small molecules has achieved great success, but most polymers are synthesized from the mixed monomers, which seriously affects batch-to-batch reproducibility. Here, a method to separate γ-Br-IC or δ-Br-IC in gram scale and apply the strategy of monomer configurational control in which two isomeric polymeric acceptors (PBTIC-γ-2F2T and PBTIC-δ-2F2T) are produced is reported. As a comparison, PBTIC-m-2F2T from the mixed monomers is also synthesized. The γ-position based polymer (PBTIC-γ-2F2T) shows good solubility and achieves the best power conversion efficiency of 14.34% with a high open-circuit voltage of 0.95 V when blended with PM6, which is among the highest values recorded to date, while the δ-position based isomer (PBTIC-δ-2F2T) is insoluble and cannot be processed after parallel polymerization. The mixed-isomers based polymer, PBTIC-m-2F2T, shows better processing capability but has a low efficiency of 3.26%. Further investigation shows that precise control of configuration helps to improve the regularity of the polymer chain and reduce the π–π stacking distance. These results demonstrate that the configurational control affords a promising strategy to achieve high-performance polymer acceptors. 相似文献